CIESC Journal

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旋转填充床内微观混合的数值模拟

梁继国;陈建峰;张建文   

  1. 北京化工大学教育部超重力工程研究中心,北京 100029;北京化工大学化学工程学院,北京 100029

  • 出版日期:2004-06-25 发布日期:2004-06-25

NUMERICAL SIMULATION OF MICROMIXING IN ROTATING PACKED BED

LIANG Jiguo;CHEN Jianfeng;ZHANG Jianwen   

  • Online:2004-06-25 Published:2004-06-25

摘要: 旋转填充床作为新型的高效反应传质设备,广泛应用于快速反应过程,如制备纳米粉体材料.对旋转填充床内微观混合进行研究,有助于进一步认识旋转填充床内高度分散液体微元在填料丝网中的流动行为和分散混合机制,为旋转填充床内液液反应混合制备纳米材料提供理论基础.基于公开文献报道的实验观测结果,通过合理假设,建立了旋转填充床内微元流动的物理模型.在该物理模型的基础上,结合此前提出的湍流混合与反应模型,模拟计算了液体微元经过实验条件下50层丝网填料最终流出填料空间的浓度分布.由浓度分布得到的微观混合特征指数与实验值进行了对比,吻合良好.

Abstract: Micromixing in the rotating packed bed(RPB) is extensively used and is a novel reactor for fast reactions such as reactive precipitation to synthesize nanoparticles. The study on micromixing in RPB is crucial in understanding the mixing-diffusion mechanism and the behavior of tiny liquid elements in the packing of RPB,which are the theoretical basis for synthesizing nanoparticles by precipitation in RPB.In this paper, on the basis of prior studies,a model describing the turbulent micromixing phenomena and reaction process in RPB is presented in accordance with the flow pattern in RPB. By sufficiently taking into account the unique characteristics of tiny liquid elements in RPB, the concentration distribution outside the packing is simulated by modifying the method proposed by the authors.The computational Xs values with the model are in reasonable agreement with the experimental results.