Effect of the Ultrasound Generated by Flat Plate Transducer Cleaning on Polluted Polyvinylidenefluoride Hollow Fiber Ultrafiltration Membrane

CIESC Journal ›› 2008, Vol. 16 ›› Issue (5): 801-804.

Effect of the Ultrasound Generated by Flat Plate Transducer Cleaning on Polluted Polyvinylidenefluoride Hollow Fiber Ultrafiltration Membrane

晋卫, 郭伟, 吕效平, 韩萍芳, 王延儒

Institute of Sonochemical Engineering, College of Chemistry and Chemical Engineering, Nanjing University of Technology, Nanjing 210009, China

收稿日期:2007-10-16 修回日期:2008-06-13 出版日期:2008-10-28 发布日期:2008-10-28
通讯作者: LÜ Xiaoping,E-mail:xplu@njut.edu.cn

Effect of the Ultrasound Generated by Flat Plate Transducer Cleaning on Polluted Polyvinylidenefluoride Hollow Fiber Ultrafiltration Membrane

JIN Wei, GUO Wei, LÜ Xiaoping, HAN Pingfang, WANG Yanru

Institute of Sonochemical Engineering, College of Chemistry and Chemical Engineering, Nanjing University of Technology, Nanjing 210009, China

Received:2007-10-16 Revised:2008-06-13 Online:2008-10-28 Published:2008-10-28

摘要/Abstract

摘要： Polyvinylidenefluoride(PVDF)hollow fiber ultrafiltration membrane is frequently employed in water treatment.However,the fouling of ultrafiltration membranes affects the economic effectiveness of such process significantly.The ultrasound generated by flat plate transducer(UFPT)was used to clean the polluted PVDF ultrafiltration membrane with 2 g·L^-1 of citric acid aqueous solution in our study.The effects of UFPT intensity on the membrane surface were studied.The new membrane was easy to be polluted by the saturated CaCl₂ solution.A synergistic effect of UFPT and 2 g·L^-1 citric acid aqueous solution could remove the foul of the membrane,and its flux could be recovered about 81%.The flux recovery of old membrane polluted was increased to 73.2% after 7 h soaking in citric acid aqueous solution,but its flux recovery without soaking was only increased to 56.2%.

关键词: ultrasound, membrane, ultrafiltration, cleaning, permeate flux

Abstract: Polyvinylidenefluoride(PVDF)hollow fiber ultrafiltration membrane is frequently employed in water treatment.However,the fouling of ultrafiltration membranes affects the economic effectiveness of such process significantly.The ultrasound generated by flat plate transducer(UFPT)was used to clean the polluted PVDF ultrafiltration membrane with 2 g·L^-1 of citric acid aqueous solution in our study.The effects of UFPT intensity on the membrane surface were studied.The new membrane was easy to be polluted by the saturated CaCl₂ solution.A synergistic effect of UFPT and 2 g·L^-1 citric acid aqueous solution could remove the foul of the membrane,and its flux could be recovered about 81%.The flux recovery of old membrane polluted was increased to 73.2% after 7 h soaking in citric acid aqueous solution,but its flux recovery without soaking was only increased to 56.2%.

Key words: ultrasound, membrane, ultrafiltration, cleaning, permeate flux

晋卫, 郭伟, 吕效平, 韩萍芳, 王延儒. Effect of the Ultrasound Generated by Flat Plate Transducer Cleaning on Polluted Polyvinylidenefluoride Hollow Fiber Ultrafiltration Membrane[J]. CIESC Journal, 2008, 16(5): 801-804.

JIN Wei, GUO Wei, LÜ Xiaoping, HAN Pingfang, WANG Yanru. Effect of the Ultrasound Generated by Flat Plate Transducer Cleaning on Polluted Polyvinylidenefluoride Hollow Fiber Ultrafiltration Membrane[J]. , 2008, 16(5): 801-804.

参考文献

1 Yan, J., Qiu, T.Q., “Advances in the ultrasound-assisted membrane-separation”, Appl. Acous., 22 (5), 45-48 (2003).
2 Huo, W.L., “Study of sonochemistry cleaning and antiscale”, J. Yulin College, 12(2), 28-30 (2002). (in Chinese) .
3 Rui, Y.N., Guo, X.H., “Research on mechanism of membrane separation process under the role of supersonic vibration”, Techniques and Equipment for Environmental Pollution Control, 3 (6), 43-46 (2002).
4 Zhang, G.J., Liu, Z.Z., “Study on assistant cleaning of ultrasound for the ultrafiltration”, Environ. Sci., 24 (6), 130-134 (2003).
5 Bao, S.H., Chen, L., “ Principle of ultrasonic cleaning and development”, Journal of Further Education of Shaanxi Normal University, 21 (2), 107-109 (2004) .
6 Chai, X.J., Kobayashi, T., Fujii, N., “Ultrasound effect on cross-flow filtration of polyacrylonitrile ultrafiltration membranes”, J. Membr. Sci., 148, 129-135 (1998).
7 Kobayashi, T., Kobayashi, T., Hosaka, Y., Fujii, N., “Ultrasound-enhanced membrane-cleaning processes applied water treatments:Influence of sonic frequency on filtration treatments”, Ultrasonics, 41,185-190 (2003).
8 Chai, X.J., Kobayashi, T., Fujii, N., “Ultrasound-associated cleaning of polymeric membranes for water treatment”, Sep. Purif. Technol., 15,139-146 (1999).
9 Li, J.X., Sanderson, R.D., Jacobs, E.P., “ Ultrasonic cleaning of nylon microfiltration membranes fouled by Kraft paper mill effluent”, J. Membr. Sci., 205, 247-257 (2002).
10 Wang, X.L., Li, X.F., “Effect of ultrasound irradiation on polymeric microfiltration membranes”, Desalination, 175, 187-196 (2005).
11 Muthukuaran, S., Kentish, S.E., Ashokkumar, M., “Mechanisams for the ultrasonic enhancement of dairy whey ultrafiltration”, J. Membr. Sci., 258, 106-114 (2005).
12 Juang, R.S., Lin, K.H., “Flux recovery in the ultrafiltration of suspended solutions with ultrasound”, J. Membr. Sci., 243, 115-124 (2004).
13 Muthukuaran, S., Kentish, S.E., Lalchandani, S., “The optimization of ultrasonic cleaning procedures for dairy fouled ultrafiltration membranes”, Ultrasonics Sonochemistry, 12, 29-35 (2005).
14 Masselin, I., Chasseray, X., “Effect of sonication on polymeric membranes”, Membr. Sci., 181, 213-220 (2001).
15 Muthukuaran, S., Yang, K., Seuren, A., “The use ultrasonic cleaning for ultrafiltration membranes in dairy industry”, Sep. Purif. Technol., 39, 99-107 (2004).

[1]	曾坚贤, 孙霞辉, 郑立锋, 贺勤程, 李书. 聚季铵盐辅助络合-超滤提取钨（VI）[J]. Chinese Journal of Chemical Engineering, 2012, 20(5): 831-836.
[2]	刘元法, 贺高红, 丁路辉, 窦红, 鞠佳, 李保军. 湍流促进器强化微滤过程的实验与CFD模拟研究[J]. Chinese Journal of Chemical Engineering, 2012, 20(4): 617-624.
[3]	伍艳辉, 谭惠芬, 李佟茗, 金源. ZSM-5填充PDMS复合膜渗透蒸发分离乙醛水溶液[J]. Chinese Journal of Chemical Engineering, 2012, 20(4): 625-632.
[4]	裴亮, 王理明, 郭维, 赵楠. 两相更新支撑液膜中金属二价镍的迁移行为研究[J]. Chinese Journal of Chemical Engineering, 2012, 20(4): 633-640.
[5]	李文军, 吴笛, 石鑫, 文利雄, 邵磊. 超声波与过氧化氢联合法降解偶氮二甲酰胺工业废水中的有机氨氮[J]. Chinese Journal of Chemical Engineering, 2012, 20(4): 754-759.
[6]	L. Chibane, B. Djellouli. 周期性输入组分和扫气在改善钯膜反应器甲烷部分氧化制氢中的作用[J]. CIESC Journal, 2012, 20(3): 577-588.
[7]	C. H. Loh, R. Wang. 添加剂和凝结剂温度对用无溶剂致相位分离法生产高性能PVDF/聚醚F127混合中空光纤膜的影响[J]. CIESC Journal, 2012, 20(1): 71-79.
[8]	刘公平, 卫旺, 金万勤, 徐南平. 陶瓷支撑的有机复合膜及其在渗透汽化中的应用[J]. CIESC Journal, 2012, 20(1): 62-70.
[9]	杨传芳. 从工业角度透视纤维介质在气溶胶过滤上的应用[J]. CIESC Journal, 2012, 20(1): 1-9.
[10]	胡纯铿, 秦晴, 高培培. Medium Optimization for Improved Ethanol Production in Very High Gravity Fermentation[J]. CIESC Journal, 2011, 19(6): 1017-1022.
[11]	陆向红, 徐之超, 计建炳. Effects of Pulse Ultrasound on Adsorption of Geniposide on Resin 1300 in a Fixed Bed[J]. CIESC Journal, 2011, 19(6): 1060-1065.
[12]	Abaji Gaikwad. Transport of Indium, Gallium and Thallium Metal Ions Through Chromatographic Fiber Supported Solid Membrane in Acetylacetone Containing Mixed Solvents[J]. CIESC Journal, 2011, 19(6): 955-963.
[13]	余从立, 刘艳梅, 陈纲领, 顾学红, 邢卫红. Pretreatment of Isopropanol Solution from Pharmaceutical Industry and Pervaporation Dehydration by NaA Zeolite Membranes[J]. CIESC Journal, 2011, 19(6): 904-910.
[14]	褚良银, 谢锐, 巨晓洁. Stimuli-responsive Membranes: Smart Tools for Controllable Mass-transfer and Separation Processes[J]. CIESC Journal, 2011, 19(6): 891-903.
[15]	吴洪, 李宪实, 聂明成, 李犇, 姜忠义. Integral PVA-PES Composite Membranes by Surface Segregation Method for Pervaporation Dehydration of Ethanol[J]. CIESC Journal, 2011, 19(5): 855-862.

Effect of the Ultrasound Generated by Flat Plate Transducer Cleaning on Polluted Polyvinylidenefluoride Hollow Fiber Ultrafiltration Membrane

Effect of the Ultrasound Generated by Flat Plate Transducer Cleaning on Polluted Polyvinylidenefluoride Hollow Fiber Ultrafiltration Membrane

PDF (PC)

可视化

被引次数

摘要/Abstract

引用本文

使用本文

参考文献

相关文章 15

编辑推荐

Metrics

本文评价