化工学报 ›› 2013, Vol. 64 ›› Issue (4): 1306-1311.DOI: 10.3969/j.issn.0438-1157.2013.04.026

• 分离工程 • 上一篇    下一篇

微细颗粒强化氧气吸收实验

姜家宗1,2, 赵博1, 曹萌1, 禚玉群1, 王淑娟1   

  1. 1. 清华大学热科学与动力工程教育部重点实验室,二氧化碳资源化利用与减排技术北京市重点实验室,北京 100084;
    2. 华北电力大学,北京102206
  • 收稿日期:2012-07-21 修回日期:2012-10-17 出版日期:2013-04-05 发布日期:2013-04-05
  • 通讯作者: 赵博
  • 作者简介:姜家宗(1982—),男,博士研究生。
  • 基金资助:

    国家自然科学基金项目(50906044)。

Fine particle enhanced oxygen absorption

JIANG Jiazong1,2, ZHAO Bo1, CAO Meng1, ZHUO Yuqun1, WANG Shujuan1   

  1. 1. Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Beijing Key Laboratory of CO2 Utilization and Reduction Technology, Tsinghua University, Beijing 100084, China;
    2. North China Electric Power University, Beijing 102206, China
  • Received:2012-07-21 Revised:2012-10-17 Online:2013-04-05 Published:2013-04-05
  • Supported by:

    supported by the National Natural Science Foundation of China(50906044).

关键词: 活性炭颗粒, 气液传质, 强制氧化, 氧气吸收

Abstract: Gas-liquid mass transfer was studied during forced sulfite oxidation in the presence of active carbon particles in a stirred tank.The influence of temperatures from 30℃ to 50℃, solid loading of fine particles from 0 to 1.0 kg·m-3, stirring speeds from 50 to 400 r·min-1, and particle sizes on average O2 gas absorption rate were studied.Experimental results show that active carbon particles could improve gas-liquid mass transfer remarkably.At 30℃, with the increase of solid loading of micro-particles, the oxygen absorption enhancement factor increases to a maximum value at the solid loading of 0.6 kg·m-3, and then decreases due to the increase of gas-liquid mass transfer resistance.For active carbon particles, the mass enhancement factor is much higher with ultrasonic processing for particle size of 1 μm.The oxygen absorption rate and absorption enhancement factor increase with the increase of stirring speed due to the acceleration of surface renewal frequency.The enhancement factor decreases as temperature increases while absorption rate increases.The result indicates that the effect of temperature on the mass transfer enhancement is stronger than the effect of fine particles.

Key words: active carbon particles, gas-liquid mass transfer, forced oxidation, oxygen absorption

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