化工学报 ›› 2022, Vol. 73 ›› Issue (10): 4298-4310.DOI: 10.11949/0438-1157.20220863

• 综述与专论 • 上一篇    下一篇

CO2光热催化还原研究进展

闫帅(), 杨海平(), 陈应泉, 王贤华, 曾阔, 陈汉平   

  1. 华中科技大学煤燃烧国家重点实验室,湖北 武汉 430074
  • 收稿日期:2022-06-21 修回日期:2022-09-06 出版日期:2022-10-05 发布日期:2022-11-02
  • 通讯作者: 杨海平
  • 作者简介:闫帅(1992—),男,博士研究生,andrewys@163.com
  • 基金资助:
    国家杰出青年科学基金项目(52125601)

Recent advances in photothermal catalysis of CO2 reduction

Shuai YAN(), Haiping YANG(), Yingquan CHEN, Xianhua WANG, Kuo ZENG, Hanping CHEN   

  1. State Key Laboratory of Coal Combustion, Huazhong University of Science and Technology, Wuhan 430074, Hubei, China
  • Received:2022-06-21 Revised:2022-09-06 Online:2022-10-05 Published:2022-11-02
  • Contact: Haiping YANG

摘要:

CO2光热催化转化是一种新型的CO2利用技术,该过程绿色、经济且无须额外能量输入,是当下的热门研究领域之一。本文主要总结了CO2光热催化转化领域的最新研究进展,介绍了基于光热转化的光热催化剂设计方法,同时从光热催化机理出发解析了CO2还原反应的光热催化剂构建策略,并揭示了CO2还原反应中的光热协同耦合机制,为光热催化剂的设计以及CO2的高效转化和利用提供参考。

关键词: CO2利用, 光热催化, 光热转化, 催化剂设计

Abstract:

Photothermal catalytic conversion of CO2 is a new type of CO2 utilization technology. The process is green, economical, and requires no additional energy input. It is one of the current hot research fields. This paper introduced recent advances in photothermal catalytic conversion of CO2 and summarized design methods for photothermal catalysts based on photo-to-thermal conversion. In addition, fabrication strategies were also investigated in the perspective of photothermal catalytic mechanism and the synergy between photo- and thermo- effects was also discussed. This work aims to promote the understanding of photothermal synergy for CO2 reduction reaction and provides reference for the design of photothermal catalysts and CO2 valorization.

Key words: CO2 utilization, photothermal catalysis, photothermal conversion, catalysts design

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