CIESC Journal ›› 2021, Vol. 72 ›› Issue (3): 1205-1216.DOI: 10.11949/0438-1157.20200921
• Reviews and monographs • Previous Articles Next Articles
WANG Ying1,2(),LI Qian3,CAO Lixia1,LI Yanxiang1,2(),LI Wangliang1,2()
Received:
2020-07-09
Revised:
2020-08-31
Online:
2021-03-05
Published:
2021-03-05
Contact:
LI Yanxiang,LI Wangliang
王莹1,2(),李倩3,曹丽霞1,李艳香1,2(),李望良1,2()
通讯作者:
李艳香,李望良
作者简介:
王莹(1994—),女,博士研究生,基金资助:
CLC Number:
WANG Ying, LI Qian, CAO Lixia, LI Yanxiang, LI Wangliang. Progress of biomass-based materials for uranium adsorption[J]. CIESC Journal, 2021, 72(3): 1205-1216.
王莹, 李倩, 曹丽霞, 李艳香, 李望良. 生物质基铀吸附材料的研究进展[J]. 化工学报, 2021, 72(3): 1205-1216.
Fig.2 (a) Time-dependent sorption behaviors of U(Ⅵ) on GO, GO-CS and GO-CS-P; (b) Effect of solution pH on the removal of U(Ⅵ) by GO, GO-CS and GO-CS-P; (c) pH-depended speciation of U(Ⅵ) in solution; (d) Sorption isotherm, Langmuir and Freundlich model fits of U(Ⅵ) on GO, GO-CS and GO-CS-P[29]
类别 | 吸附剂名称 | 吸附条件 | 最高吸附量/(mg·g-1) | 文献 |
---|---|---|---|---|
壳聚糖颗粒 | 戊二醛和硫脲交联磁性壳聚糖(TTG-MCTS) | C0 = 40 ~ 140 mg·L-1 pH = 5.00,0.60 g·L-1 | 161.3 | [ |
二乙烯三胺五乙酸功能化磁性壳聚糖(DTPA-MCS) | C0 = 10 ~ 100 mg·L-1 pH = 5.00,0.40 g·L-1 | 178.20 | [ | |
三聚磷酸钠交联磁性壳聚糖树脂(TPP-MCR) | C0 = 40 ~ 150 mg·L-1 pH = 3.00,0.40 g·L-1 | 166.70 | [ | |
离子印迹磁性壳聚糖微球(IMCR) | C0 = 15 ~ 420 mg·L-1 pH = 5.00,1.00 g·L-1 | 187.26 | [ | |
壳聚糖纤维 | 共混纤维吸附剂(PVP/CS fibers) | C0 = 1~ 270 mg·L-1 pH = 6.00,1.00 g·L-1 | 167±25 | [ |
壳聚糖纤维膜(CS-80%) | C0 = 10 ~ 100 mg·L-1 pH = 5.00,0.50 g·L-1 | 196.74 | [ | |
壳聚糖复合材料 | 壳聚糖/氧化石墨烯复合材料(CS/GO) | C0 = 2 ~ 100 mg·L-1 pH = 5.00,0.15 g·L-1 | 217.40 | [ |
多巴胺交联氧化石墨烯/壳聚糖气凝胶(GO@PDA/CS) | C0 = 10 ~ 220 mg·L-1 pH = 6.00,0.30 g·L-1 | 415.90 | [ | |
磷酸化的氧化石墨烯/壳聚糖复合材料(GO-CS-P) | C0 = 2 ~ 140 mg·L-1 pH = 5.00,0.05 g·L-1 | 779.44 | [ | |
磷酸化壳聚糖/羧甲基纤维素复合材料(CSP-CMCP) | C0 = 10 ~ 120 mg·L-1 pH = 5.00,0.05 g·L-1 | 977.54 | [ | |
壳聚糖-氧化石墨烯/ZIF泡沫吸附剂(GCZ8A) | C0 = 2 ~ 120 mg·L-1 pH = 8.00,0.20 g·L-1 | 361.01 | [ |
Table 1 Summarizes of chitosan-based materials and uranium adsorption abilities
类别 | 吸附剂名称 | 吸附条件 | 最高吸附量/(mg·g-1) | 文献 |
---|---|---|---|---|
壳聚糖颗粒 | 戊二醛和硫脲交联磁性壳聚糖(TTG-MCTS) | C0 = 40 ~ 140 mg·L-1 pH = 5.00,0.60 g·L-1 | 161.3 | [ |
二乙烯三胺五乙酸功能化磁性壳聚糖(DTPA-MCS) | C0 = 10 ~ 100 mg·L-1 pH = 5.00,0.40 g·L-1 | 178.20 | [ | |
三聚磷酸钠交联磁性壳聚糖树脂(TPP-MCR) | C0 = 40 ~ 150 mg·L-1 pH = 3.00,0.40 g·L-1 | 166.70 | [ | |
离子印迹磁性壳聚糖微球(IMCR) | C0 = 15 ~ 420 mg·L-1 pH = 5.00,1.00 g·L-1 | 187.26 | [ | |
壳聚糖纤维 | 共混纤维吸附剂(PVP/CS fibers) | C0 = 1~ 270 mg·L-1 pH = 6.00,1.00 g·L-1 | 167±25 | [ |
壳聚糖纤维膜(CS-80%) | C0 = 10 ~ 100 mg·L-1 pH = 5.00,0.50 g·L-1 | 196.74 | [ | |
壳聚糖复合材料 | 壳聚糖/氧化石墨烯复合材料(CS/GO) | C0 = 2 ~ 100 mg·L-1 pH = 5.00,0.15 g·L-1 | 217.40 | [ |
多巴胺交联氧化石墨烯/壳聚糖气凝胶(GO@PDA/CS) | C0 = 10 ~ 220 mg·L-1 pH = 6.00,0.30 g·L-1 | 415.90 | [ | |
磷酸化的氧化石墨烯/壳聚糖复合材料(GO-CS-P) | C0 = 2 ~ 140 mg·L-1 pH = 5.00,0.05 g·L-1 | 779.44 | [ | |
磷酸化壳聚糖/羧甲基纤维素复合材料(CSP-CMCP) | C0 = 10 ~ 120 mg·L-1 pH = 5.00,0.05 g·L-1 | 977.54 | [ | |
壳聚糖-氧化石墨烯/ZIF泡沫吸附剂(GCZ8A) | C0 = 2 ~ 120 mg·L-1 pH = 8.00,0.20 g·L-1 | 361.01 | [ |
Fig.3 (a) The uranium adsorption capacity at different pH (C0 = 10 mg·L-1, V = 100 ml, sorbent dose (SD) = 0.03 g, time =8 h); (b) The uranium adsorption capacity at different initial concentration (V = 100 ml, SD = 0.03 g, pH = 5, time =8 h); (c) The experimental data and fitting curves of adsorption isotherms (V = 100 ml, SD = 0.03 g, pH = 5, time =8 h); (d) The experimental data and fitting curves of adsorption kinetics (V = 100 ml, SD = 0.03 g, pH = 5) (the counter ions of uranium were hydroxyl) [50]
吸附剂 | 吸附条件 | 最高吸附量/(mg·g-1) | 自然/模拟海水提铀 | 文献 |
---|---|---|---|---|
丝瓜络 (LC-PAA-PEI) | C0 = 50 ~ 350 mg·L-1 pH = 6.00,0.40 g·L-1 | 444.40 | R>90% | [ |
大麻纤维 (HF-PE1-GDAC) | C0 = 5 ~ 400 mg·L-1 pH = 7.00,0.40 g·L-1 | 414.93 | R=71% | [ |
剑麻纤维 (ATMP-Sisal-150) | C0 = 10 mg·L-1 模拟海水 | 16 | 0.10 mg·g-1 自然海水 | [ |
纤维素纤维 (PAO-CFs) | C0 = 2 ~ 18 mg·L-1 pH = 5.00,0.30 g·L-1 | 52.88 | 1.22 mg U·(g Ads)-1 | [ |
Table 2 Summarizes of cellulose-based materials used for uranium extraction from seawater
吸附剂 | 吸附条件 | 最高吸附量/(mg·g-1) | 自然/模拟海水提铀 | 文献 |
---|---|---|---|---|
丝瓜络 (LC-PAA-PEI) | C0 = 50 ~ 350 mg·L-1 pH = 6.00,0.40 g·L-1 | 444.40 | R>90% | [ |
大麻纤维 (HF-PE1-GDAC) | C0 = 5 ~ 400 mg·L-1 pH = 7.00,0.40 g·L-1 | 414.93 | R=71% | [ |
剑麻纤维 (ATMP-Sisal-150) | C0 = 10 mg·L-1 模拟海水 | 16 | 0.10 mg·g-1 自然海水 | [ |
纤维素纤维 (PAO-CFs) | C0 = 2 ~ 18 mg·L-1 pH = 5.00,0.30 g·L-1 | 52.88 | 1.22 mg U·(g Ads)-1 | [ |
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