CIESC Journal ›› 2023, Vol. 74 ›› Issue (2): 599-616.DOI: 10.11949/0438-1157.20221088
• Reviews and monographs • Previous Articles Next Articles
Min LI1,2,3(), Xueru YAN1,2,3, Xinlei LIU1,2,3()
Received:
2022-10-09
Revised:
2022-12-01
Online:
2023-03-21
Published:
2023-02-05
Contact:
Xinlei LIU
李敏1,2,3(), 阎雪茹1,2,3, 刘新磊1,2,3()
通讯作者:
刘新磊
作者简介:
李敏(1998—),女,硕士研究生,limin1013@tju.edu.cn
基金资助:
CLC Number:
Min LI, Xueru YAN, Xinlei LIU. Advances in benzimidazole-linked polymer adsorbents and membranes[J]. CIESC Journal, 2023, 74(2): 599-616.
李敏, 阎雪茹, 刘新磊. 苯并咪唑连接聚合物吸附剂和膜研究进展[J]. 化工学报, 2023, 74(2): 599-616.
聚合物 | SABET①/(m2/g) | 吸附量②/(mg/g) | 选择性③ | 文献 | |||
---|---|---|---|---|---|---|---|
CO2 at 1 bar | N2 at 1 bar | CH4 at 1 bar | CO2/N2 | CO2/CH4 | |||
BILP-1 | 1172 | 188(131) | 5.0(7.3) | 23(16) | 70(36) | 10(7) | [ |
BILP-2 | 708 | 149(104) | 3.4(2.5) | 14(9) | 113(71) | 17(12) | [ |
BILP-3 | 1306 | 225(145) | 3.3(2.4) | 24(17) | 59(31) | 8(5) | [ |
BILP-4 | 1135 | 235(158) | 1.1(3.8) | 26(18) | 79(32) | 10(7) | [ |
BILP-5 | 599 | 128(87) | 0.2(2.7) | 15(10) | 95(36) | 10(6) | [ |
BILP-6 | 1261 | 211(121) | 6.8(6.7) | 27(19) | 63(39) | 8(5) | [ |
BILP-6-NH2 | 1185 | 244.8(164.7) | — | — | — | —(8.4) | [ |
BILP-7 | 1122 | 193(122) | 5.63(5.40) | 19(12) | 62(34) | 9(7) | [ |
BILP-10 | 787 | 177(111) | — | 16(11) | 111(59) | 14(7) | [ |
BILP-11 | 658 | 136(88) | — | 16(10) | 103(55) | 11(7) | [ |
BILP-12 | 1497 | 223(140) | — | 24(15) | 56(31) | 8(6) | [ |
BILP-13 | 677 | 113(79) | — | 12(9) | 103(38) | 9(6) | [ |
BILP-14 | 1005 | 170(—) | — | — | 56(49) | 10(9) | [ |
BILP-15 | 448 | 118(80) | 5.7(3.8) | 13.5(7.2) | 83(63) | 9(8) | [ |
BILP-16 | 435 | 118.7(80.7) | 6.5(4.3) | 13.5(8.0) | 53(49) | 10(8) | [ |
BILP-15(AC) | 862 | 151(101) | 7.2(5.8) | 16.4(10.3) | 61(50) | 9(7) | [ |
BILP-16(AC) | 643 | 152(102.2) | 8.0(4.8) | 17.4(10.3) | 49(61) | 9(7) | [ |
BILP-17 | 952 | — | — | — | — | — | [ |
BILP-18 | 947 | — | — | — | — | — | [ |
BILP-19 | 144 | 2630.95bar(229) | —(3) | 14.1(8.2) | —(59.1) | 11.9(12.3) | [ |
BILP-101 | —(1070.15bar) | — | — | —(80) | — | [ | |
PPN-101 | 226.2(—) | — | — | 199(—) | — | [ | |
IBFNP-1 | 232(148) | — | — | 65(44) | 11(8) | [ | |
IBLP | 48.06 | 46.5(30.7) | — | — | — | — | [ |
IBLP-600 | 161.06 | 85.1(59.9) | — | — | — | — | [ |
IBLP-700 | 270.64 | 121.8(90.7) | — | — | — | — | [ |
IBLP-800 | 339 | 130.4(98.4) | — | — | — | — | [ |
BINP-1 | 64 | 7.8(—) | — | — | — | — | [ |
BINP-2 | 32 | 7(—) | — | — | — | — | [ |
TBILP-1 | 330 | 117(78) | — | — | —(63) | —(9) | [ |
TBILP-2 | 1080 | 228(146) | — | — | —(40) | —(7) | [ |
CTF-BI-3 | 677 | 77.51.1bar(—) | 1.4(—) | — | 88.5(—) | — | [ |
CTF-BI-4 | 1025 | 108.7(—) | 7.1(—) | — | 44.0(—) | — | [ |
CTF-BI-5 | 836 | 100.6(—) | 6.9(—) | — | 35.6(—) | — | [ |
CTF-BI-6 | 759 | 75.2(—) | 6.3(—) | — | 34.5(—) | — | [ |
CTF-BI-7 | 642 | 56.3(—) | 5.3(—) | — | 39.7(—) | — | [ |
CTF-BI-9 | 885 | 96.1(—) | 5.4(—) | — | 67.4(—) | — | [ |
CTF-BI-10 | 1099 | 99.9(—) | 9.0(—) | — | 31.3(—) | — | [ |
CTF-BI-11 | 1549 | 110.5(—) | 9.6(—) | — | 34.3(—) | — | [ |
CTF-BIB-1 | 97.6(56.8) | 10.3(5.1) | 30.3(16.2) | 29.3(—) | 6.8(—) | [ | |
CTF-BIB-2 | 1714 | 92.3(55.6) | 10.0(5.3) | 31.9(17.5) | 33.1(—) | 7.3(—) | [ |
CTF-BIB-3 | 2088 | 86.4(48.5) | 9.8(3.9) | 27.3(16.2) | 21.2(—) | 4.7(—) | [ |
CTF-DI-2 | 420 | 33.5(19.3) | — | — | 35(—) | 14(—) | [ |
CTF-DI-3 | 1877 | 80.4(44.7) | — | — | 26(—) | 6(—) | [ |
CTF-DI-4 | 1769 | 67.6(39.3) | — | — | 42(—) | 8(—) | [ |
CTF-DI-5 | 1207 | 50.9(29.4) | — | — | 27(—) | 6(—) | [ |
CTF-DI-6 | 697 | 62.8(40.0) | — | — | 53(—) | 15(—) | [ |
CTF-DI-7 | 1300 | 89.2(54.2) | — | — | 41(—) | 11(—) | [ |
CTF-DI-8 | 1749 | 77.8(44.5) | — | — | 35(—) | 8(—) | [ |
CTF-DI-9 | 1228 | 59.7(35.4) | — | — | 14(—) | 6(—) | [ |
PBILP | 121.4(79.2) | — | — | 72(—) | 7.2(—) | [ |
Table 1 BET surface area, gas uptake and selectivity (CO2/N2 and CO2/CH4) of benzimidazole-linked polymers
聚合物 | SABET①/(m2/g) | 吸附量②/(mg/g) | 选择性③ | 文献 | |||
---|---|---|---|---|---|---|---|
CO2 at 1 bar | N2 at 1 bar | CH4 at 1 bar | CO2/N2 | CO2/CH4 | |||
BILP-1 | 1172 | 188(131) | 5.0(7.3) | 23(16) | 70(36) | 10(7) | [ |
BILP-2 | 708 | 149(104) | 3.4(2.5) | 14(9) | 113(71) | 17(12) | [ |
BILP-3 | 1306 | 225(145) | 3.3(2.4) | 24(17) | 59(31) | 8(5) | [ |
BILP-4 | 1135 | 235(158) | 1.1(3.8) | 26(18) | 79(32) | 10(7) | [ |
BILP-5 | 599 | 128(87) | 0.2(2.7) | 15(10) | 95(36) | 10(6) | [ |
BILP-6 | 1261 | 211(121) | 6.8(6.7) | 27(19) | 63(39) | 8(5) | [ |
BILP-6-NH2 | 1185 | 244.8(164.7) | — | — | — | —(8.4) | [ |
BILP-7 | 1122 | 193(122) | 5.63(5.40) | 19(12) | 62(34) | 9(7) | [ |
BILP-10 | 787 | 177(111) | — | 16(11) | 111(59) | 14(7) | [ |
BILP-11 | 658 | 136(88) | — | 16(10) | 103(55) | 11(7) | [ |
BILP-12 | 1497 | 223(140) | — | 24(15) | 56(31) | 8(6) | [ |
BILP-13 | 677 | 113(79) | — | 12(9) | 103(38) | 9(6) | [ |
BILP-14 | 1005 | 170(—) | — | — | 56(49) | 10(9) | [ |
BILP-15 | 448 | 118(80) | 5.7(3.8) | 13.5(7.2) | 83(63) | 9(8) | [ |
BILP-16 | 435 | 118.7(80.7) | 6.5(4.3) | 13.5(8.0) | 53(49) | 10(8) | [ |
BILP-15(AC) | 862 | 151(101) | 7.2(5.8) | 16.4(10.3) | 61(50) | 9(7) | [ |
BILP-16(AC) | 643 | 152(102.2) | 8.0(4.8) | 17.4(10.3) | 49(61) | 9(7) | [ |
BILP-17 | 952 | — | — | — | — | — | [ |
BILP-18 | 947 | — | — | — | — | — | [ |
BILP-19 | 144 | 2630.95bar(229) | —(3) | 14.1(8.2) | —(59.1) | 11.9(12.3) | [ |
BILP-101 | —(1070.15bar) | — | — | —(80) | — | [ | |
PPN-101 | 226.2(—) | — | — | 199(—) | — | [ | |
IBFNP-1 | 232(148) | — | — | 65(44) | 11(8) | [ | |
IBLP | 48.06 | 46.5(30.7) | — | — | — | — | [ |
IBLP-600 | 161.06 | 85.1(59.9) | — | — | — | — | [ |
IBLP-700 | 270.64 | 121.8(90.7) | — | — | — | — | [ |
IBLP-800 | 339 | 130.4(98.4) | — | — | — | — | [ |
BINP-1 | 64 | 7.8(—) | — | — | — | — | [ |
BINP-2 | 32 | 7(—) | — | — | — | — | [ |
TBILP-1 | 330 | 117(78) | — | — | —(63) | —(9) | [ |
TBILP-2 | 1080 | 228(146) | — | — | —(40) | —(7) | [ |
CTF-BI-3 | 677 | 77.51.1bar(—) | 1.4(—) | — | 88.5(—) | — | [ |
CTF-BI-4 | 1025 | 108.7(—) | 7.1(—) | — | 44.0(—) | — | [ |
CTF-BI-5 | 836 | 100.6(—) | 6.9(—) | — | 35.6(—) | — | [ |
CTF-BI-6 | 759 | 75.2(—) | 6.3(—) | — | 34.5(—) | — | [ |
CTF-BI-7 | 642 | 56.3(—) | 5.3(—) | — | 39.7(—) | — | [ |
CTF-BI-9 | 885 | 96.1(—) | 5.4(—) | — | 67.4(—) | — | [ |
CTF-BI-10 | 1099 | 99.9(—) | 9.0(—) | — | 31.3(—) | — | [ |
CTF-BI-11 | 1549 | 110.5(—) | 9.6(—) | — | 34.3(—) | — | [ |
CTF-BIB-1 | 97.6(56.8) | 10.3(5.1) | 30.3(16.2) | 29.3(—) | 6.8(—) | [ | |
CTF-BIB-2 | 1714 | 92.3(55.6) | 10.0(5.3) | 31.9(17.5) | 33.1(—) | 7.3(—) | [ |
CTF-BIB-3 | 2088 | 86.4(48.5) | 9.8(3.9) | 27.3(16.2) | 21.2(—) | 4.7(—) | [ |
CTF-DI-2 | 420 | 33.5(19.3) | — | — | 35(—) | 14(—) | [ |
CTF-DI-3 | 1877 | 80.4(44.7) | — | — | 26(—) | 6(—) | [ |
CTF-DI-4 | 1769 | 67.6(39.3) | — | — | 42(—) | 8(—) | [ |
CTF-DI-5 | 1207 | 50.9(29.4) | — | — | 27(—) | 6(—) | [ |
CTF-DI-6 | 697 | 62.8(40.0) | — | — | 53(—) | 15(—) | [ |
CTF-DI-7 | 1300 | 89.2(54.2) | — | — | 41(—) | 11(—) | [ |
CTF-DI-8 | 1749 | 77.8(44.5) | — | — | 35(—) | 8(—) | [ |
CTF-DI-9 | 1228 | 59.7(35.4) | — | — | 14(—) | 6(—) | [ |
PBILP | 121.4(79.2) | — | — | 72(—) | 7.2(—) | [ |
聚合物 | 电导率 σ/( | 温度 T/K | 湿度 RH/% | 活化能 Ea/eV | 文献 |
---|---|---|---|---|---|
DPBIB | 9.3 | 393 | 100 | — | [ |
PON-4 | 9.7 | 393 | 0 | 0.6 | [ |
PON-5 | 2.0 | 393 | 0 | 0.36 | [ |
PON-6 | 4.9 | 393 | 0 | 0.46 | [ |
BIP | 3.2 | 368 | 95 | 0.34 | [ |
BILP-10 | 1.2 | 368 | 95 | — | [ |
2.4 | 393 | 0 | 0.16 | [ | |
H3PO4@TPB-DABI-COF[66%(质量分数)] | 1.52 | 433 | 0 | 0.17 | [ |
Nafion 112 | 9.4 | 393 | 100 | — | [ |
Nafion 115 | 1.3 | 363 | 100 | — | [ |
Nafion 117 | 4.5 | 383 | 0 | — | [ |
Table 2 Proton conductivity of benzimidazole-linked polymers and commercial Nafion membranes
聚合物 | 电导率 σ/( | 温度 T/K | 湿度 RH/% | 活化能 Ea/eV | 文献 |
---|---|---|---|---|---|
DPBIB | 9.3 | 393 | 100 | — | [ |
PON-4 | 9.7 | 393 | 0 | 0.6 | [ |
PON-5 | 2.0 | 393 | 0 | 0.36 | [ |
PON-6 | 4.9 | 393 | 0 | 0.46 | [ |
BIP | 3.2 | 368 | 95 | 0.34 | [ |
BILP-10 | 1.2 | 368 | 95 | — | [ |
2.4 | 393 | 0 | 0.16 | [ | |
H3PO4@TPB-DABI-COF[66%(质量分数)] | 1.52 | 433 | 0 | 0.17 | [ |
Nafion 112 | 9.4 | 393 | 100 | — | [ |
Nafion 115 | 1.3 | 363 | 100 | — | [ |
Nafion 117 | 4.5 | 383 | 0 | — | [ |
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