doi:10.11949/0438-1157.20190698

Abstract

Abstract:

As a basic form of the substance, plasma is different from solid, liquid and gas due to its unique high activity. It has gradually been applied in many fields and has developed into a new discipline. The gas-liquid chemical reaction involving the non-thermal plasma could generate more reactive oxygen species, and the fluidity of liquid could enhance the mass transfer in the gas-liquid non-thermal plasma reactors. So, the reaction of non-thermal plasma generated by the gas discharge and liquid phase has an important application value in many fields. The discharge patterns and characterization techniques of various non-thermal plasmas are reviewed. Furthermore, the different structures and applications of gas-liquid non-thermal plasma multiphase reactors are highlighted, and then the development of gas-liquid non-thermal plasma is prospected.

Key words: non-thermal plasma, gas-liquid two-phase flow, multiphase reactor, mass transfer, gas-liquid reaction

摘要：

等离子体作为物质存在的一种基本形态，因其特有的高活性而不同于固、液、气三种形态，逐渐应用于多个领域，并发展成了一门新兴学科。由于冷等离子体参与的气液化学反应能产生更多的活性物质，而且液体的流动性能够强化活性物质的传递，因此，气体放电产生的冷等离子体与液相反应在许多领域表现出重要的应用价值，更具有探究意义。综述了几种冷等离子体的放电形式以及表征技术，重点阐述了气液冷等离子体多相反应器的不同结构以及应用，并对气液冷等离子体技术发展进行了展望。

关键词: 冷等离子体, 气液两相流, 多相反应器, 传质, 气液反应

CLC Number:

TQ 028.8

Yong CAI, Chuang LIANG, Yong LUO, Guangwen CHU, Mengjun SU, Baochang SUN, Jianfeng CHEN. [J]. CIESC Journal, 2019, 70(10): 3847-3858.

蔡勇, 梁闯, 罗勇, 初广文, 苏梦军, 孙宝昌, 陈建峰. 气液冷等离子体多相反应器基础研究与应用进展[J]. 化工学报, 2019, 70(10): 3847-3858.

Figures/Tables 7

Fig.1 Schematic drawing of reactive-PLIF measurement equipment(a), diagram of concentration field distribution(b), temporally averaged emission spectra observed in oxygen discharge(c)

Fig.2 Gas-liquid stratified non-thermal plasma reactor

Fig.3 Bubbling non-thermal plasma reactor

Fig.4 Spray non-thermal plasma reactor

Fig.5 Relative energy efficiencies of gas-liquid non-thermal plasma reactors for decomposing toxic organic compounds in water

Fig.6 Energy efficiency comparisons of various plasma reactors

Fig.7 Penetration depth of various reactive species

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气液冷等离子体多相反应器基础研究与应用进展

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