CIESC Journal ›› 2020, Vol. 71 ›› Issue (11): 4851-4872.DOI: 10.11949/0438-1157.20201296
• Celebration Column for School of Chemistry and Chemical Engineering, Nanjing University • Previous Articles Next Articles
Jie ZHAO1(),Yue GUO1,Zhen SHEN1,Lijun YANG1,Qiang WU1(
),Xizhang WANG1,Zheng HU1,2(
)
Received:
2020-09-09
Revised:
2020-09-17
Online:
2020-11-05
Published:
2020-11-05
Contact:
Qiang WU,Zheng HU
赵杰1(),郭月1,沈桢1,杨立军1,吴强1(
),王喜章1,胡征1,2(
)
通讯作者:
吴强,胡征
作者简介:
赵杰(1987—),男,博士研究生,基金资助:
CLC Number:
Jie ZHAO,Yue GUO,Zhen SHEN,Lijun YANG,Qiang WU,Xizhang WANG,Zheng HU. Research progress of high-rate capacity layered double hydroxide supercapacitor materials[J]. CIESC Journal, 2020, 71(11): 4851-4872.
赵杰,郭月,沈桢,杨立军,吴强,王喜章,胡征. 高倍率容量层状双金属氢氧化物超级电容材料的研究进展[J]. 化工学报, 2020, 71(11): 4851-4872.
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Fig.4 Ragone plot for various electrical energy storage devices[126](performances of supercapacitors in Ref. [33-34,46,93,97,106,109,120-123,125] are also provided for comparison, the time constants of the devices are marked in the figure)
Fig.5 Characterization of the monolayer NiTi-LDH nanosheets[36]: TEM image (a); HRTEM image (b); AFM image(c) and the corresponding height profiles (d) (profiles of 1—3 in Fig.(d) correspond to the nanosheets of 1—3 in Fig. (c))
Fig.6 Hierarchical NiAl-LDH and rate capacities[39]: schematic preparation (a), core-shell structure[(b),(c)], yolk-shell structure[(d),(e)], hollow structure[(f),(g)], nanoparticles (h), rate capacities (i)
Fig.7 Influence of hierarchical structure on rate capacity of the CoAl-LDH nanosheet array[43]: schematic diagram of P-CO3-LDH and H-CO3-LDH (a), rate capacities (b) (performance of H-OH-LDH in Fig. (b) is provided for reference)
Fig.8 Electrochemical performances of the CoAl-LDH and the CoAl-LDH/CNTs composite[46]: schematic preparation of the CoAl-LDH/CNTs composite (a), electrochemical impedance spectra (b) (Rs is the intrinsic Ohmic resistance, Rct is the charge transfer resistance), rate capacities(c) ( in Fig. (b),(c) , the data of CNTs are also presented for reference)
Fig.9 Electrochemical performances of the NiAl-LDH and the NiAl-LDH/rGO composite[58]: schematic preparation of the NiAl-LDH/rGO composite (a), electrochemical impedance spectra (b), rate capacities at 3.57—17.86 A·g-1 (c)
Fig.10 Electrochemical performances of CC-LDH and CC-NC-LDH electrodes[93]: schematic preparation of the CC-NC-LDH electrode (a), electrochemical impedance spectra (b), rate capacities (c) (the performance of NiCo-LDH in Fig.(c) is also presented for reference)
Fig.12 Influence of interlayer distance on rate capacity of CoAl-LDH[109]: schematic regulation of the interlayer distance (a), electrochemical impedance spectra (b), rate capacities at 1—32 A·g-1(c) ( DS- is dodecyl sulfate anion in Ref.[109])
Fig.13 Schematic preparation of the LDHs-based composites by exfoliation-self-assembly method: CoAl-LDH/rGO film (a) [120],CoNi-LDH/PEDOT:PSS composite (b) [122]
Fig.14 The regulation of interlayer distance of NiAl-LDH nanosheet arrays and the related electrochemical performances[124]: schematic regulation of the interlayer distance(a), electrochemical impedance spectra(b), rate capacities(c)(in Fig.(c), DS is dodecanesulfonate anion. PS is 1-pentanesulfonate anion)
Fig.15 Influences of the interlayer distance on RESR and rate capacity in NiCo-LDH[125]: schematic regulation of interlayer distance(a), RESR(b) and rate capacities(c) of the straight-chain anions intercalated LDHs, RESR (d) and rate capacities(e) of the conjugated-plane anions intercalated LDHs
Sample | Capacitance/(F·g-1) | Ref. | Sample | Capacitance/(F·g-1) | Ref. | ||
---|---|---|---|---|---|---|---|
at low current (≤ 50 A·g-1) | at high current (> 50 A·g-1) | at low current (≤ 50 A·g-1) | at high current (> 50 A·g-1) | ||||
regulating compositions | depositing/growing on conductive substrates | ||||||
NiCoAl-LDH | 2062 (1) 553 (20) | ― | [ | CoAl-LDH/CC | 616.9 (1) 454.4 (20) | ― | [ |
CoNi-LDH | 2614 (5) | ― | [ | NiCo-LDH/ N-doped CC | 1817 (1) | 1092 (100) | [ |
CoⅡCoⅢ-LDH | 715 (0.5) 130 (50) | ― | [ | CoMn-LDH/CC | 1079 (2.1) 891 (42) | ― | [ |
amorphizating | NiCo-LDH/CC | 1927 (2) 1546 (30) | ― | [ | |||
NiCoMn-LDHs | 1440 (1) 1104 (50) | ― | [ | NiCo-LDH/CC | 2105 (2) 1191.3 (20) | ― | [ |
nanostructuring | NiCo-LDH/NF | 2682 (3) 1706 (20) | ― | [ | |||
NiTi-LDH | 2310 (1.5) 1206 (30) | ― | [ | MnCo-LDHs@ Ni(OH)2/NF | 2320 (3) 1308 (30) | ― | [ |
constructing hierarchical structures | NiMn-LDH/NF | 1511 (2.5) 1210 (48) | ― | [ | |||
NiAl-LDH | 735 (2) 548 (25) | ― | [ | NiCo-LDH/NF | 2184 (1) 1494 (20) | ― | [ |
NiCo-LDH | 2275.5 (1) 1007.8 (25) | ― | [ | NiCo-LDH/SS | 2104 (1) | ― | [ |
NiCo-LDH | 1887.5 (1) 1187.5 (10) | ― | [ | expanding interlayer distance | |||
NiFe-LDH | 1061 (1) 598 (10) | ― | [ | CoFe-LDH | 456 (2) 337 (20) | ― | [ |
CoAl-LDH | 1031 (1) 763 (40) | 680 (100) | [ | CoAl-LDH | 1481.7 (1) 856.7 (32) | ― | [ |
compositing with carbon | NiCo-LDH | 1646 (3) 680 (10) | ― | [ | |||
NiCo-LDH/CNTs | 1843 (0.5) 1231 (10) | ― | [ | CoAl-LDH | 1100 (1) 750 (30) | ― | [ |
NiAl-LDH/CNTs | 2034 (1) 1729 (10) | ― | [ | CoⅡCoⅢ-LDH | 1055 (1) 300 (15) | ― | [ |
NiMn-LDH/CNTs | 2960 (1.5) 2353 (30) | ― | [ | NiMn-LDH | 1881 (1) 649 (10) | ― | [ |
NiCo-LDH/CNTs | 1896 (1) 1479 (40) | ― | [ | NiCo-LDH | 1580 (10) | ― | [ |
CoAl-LDH/CNTs | 1949.5 (1) 1066.4 (10) | ― | [ | CoⅡCoⅢ-LDH | 590 (10) | ― | [ |
NiCoAl-LDH/rGO | 1866 (1) 1360 (10) | ― | [ | selective etching | |||
NiAl-LDH/rGO | 2712.7 (1) 1174 (50) | ― | [ | NiCoAl-LDH | 1289 (1) 738 (30) | ― | [ |
NiCo-LDH/rGO | 1911.1 (2) 1469.8 (20) | ― | [ | exfoliation-self-assembly | |||
MgAl-LDH/rGO | 1334 (1) | ― | [ | CoAl-LDH/rGO | 1043 (1) 912 (20) | ― | [ |
CoMn-LDH/rGO | 1635 (1) 1161 (10) | ― | [ | CoNi-LDH/ PEDOT:PSS | 960 (2) 804 (30) | ― | [ |
NiCoAl-LDH/rGO | 1544 (1) 1081 (40) | ― | [ | depositing/growing on conductive substrates+ expanding interlayer distance | |||
NiAl-LDH/NF | 1125 (1) | 819 (200) | [ | ||||
NiFe-LDH/rGO | 1196 (1) 861 (10) | ― | [ | sub-nanometer-scale fine regulation of interlayer distance | |||
NiCo-LDH/C | 2558 (1) 1916 (20) | ― | [ | NiCo-LDH | 2115 (1) 949 (50) | 626 (100) 410 (150) | [ |
Table 1 Rate capacities of LDHs-based electrode materials in each strategy (three-electrode test system)
Sample | Capacitance/(F·g-1) | Ref. | Sample | Capacitance/(F·g-1) | Ref. | ||
---|---|---|---|---|---|---|---|
at low current (≤ 50 A·g-1) | at high current (> 50 A·g-1) | at low current (≤ 50 A·g-1) | at high current (> 50 A·g-1) | ||||
regulating compositions | depositing/growing on conductive substrates | ||||||
NiCoAl-LDH | 2062 (1) 553 (20) | ― | [ | CoAl-LDH/CC | 616.9 (1) 454.4 (20) | ― | [ |
CoNi-LDH | 2614 (5) | ― | [ | NiCo-LDH/ N-doped CC | 1817 (1) | 1092 (100) | [ |
CoⅡCoⅢ-LDH | 715 (0.5) 130 (50) | ― | [ | CoMn-LDH/CC | 1079 (2.1) 891 (42) | ― | [ |
amorphizating | NiCo-LDH/CC | 1927 (2) 1546 (30) | ― | [ | |||
NiCoMn-LDHs | 1440 (1) 1104 (50) | ― | [ | NiCo-LDH/CC | 2105 (2) 1191.3 (20) | ― | [ |
nanostructuring | NiCo-LDH/NF | 2682 (3) 1706 (20) | ― | [ | |||
NiTi-LDH | 2310 (1.5) 1206 (30) | ― | [ | MnCo-LDHs@ Ni(OH)2/NF | 2320 (3) 1308 (30) | ― | [ |
constructing hierarchical structures | NiMn-LDH/NF | 1511 (2.5) 1210 (48) | ― | [ | |||
NiAl-LDH | 735 (2) 548 (25) | ― | [ | NiCo-LDH/NF | 2184 (1) 1494 (20) | ― | [ |
NiCo-LDH | 2275.5 (1) 1007.8 (25) | ― | [ | NiCo-LDH/SS | 2104 (1) | ― | [ |
NiCo-LDH | 1887.5 (1) 1187.5 (10) | ― | [ | expanding interlayer distance | |||
NiFe-LDH | 1061 (1) 598 (10) | ― | [ | CoFe-LDH | 456 (2) 337 (20) | ― | [ |
CoAl-LDH | 1031 (1) 763 (40) | 680 (100) | [ | CoAl-LDH | 1481.7 (1) 856.7 (32) | ― | [ |
compositing with carbon | NiCo-LDH | 1646 (3) 680 (10) | ― | [ | |||
NiCo-LDH/CNTs | 1843 (0.5) 1231 (10) | ― | [ | CoAl-LDH | 1100 (1) 750 (30) | ― | [ |
NiAl-LDH/CNTs | 2034 (1) 1729 (10) | ― | [ | CoⅡCoⅢ-LDH | 1055 (1) 300 (15) | ― | [ |
NiMn-LDH/CNTs | 2960 (1.5) 2353 (30) | ― | [ | NiMn-LDH | 1881 (1) 649 (10) | ― | [ |
NiCo-LDH/CNTs | 1896 (1) 1479 (40) | ― | [ | NiCo-LDH | 1580 (10) | ― | [ |
CoAl-LDH/CNTs | 1949.5 (1) 1066.4 (10) | ― | [ | CoⅡCoⅢ-LDH | 590 (10) | ― | [ |
NiCoAl-LDH/rGO | 1866 (1) 1360 (10) | ― | [ | selective etching | |||
NiAl-LDH/rGO | 2712.7 (1) 1174 (50) | ― | [ | NiCoAl-LDH | 1289 (1) 738 (30) | ― | [ |
NiCo-LDH/rGO | 1911.1 (2) 1469.8 (20) | ― | [ | exfoliation-self-assembly | |||
MgAl-LDH/rGO | 1334 (1) | ― | [ | CoAl-LDH/rGO | 1043 (1) 912 (20) | ― | [ |
CoMn-LDH/rGO | 1635 (1) 1161 (10) | ― | [ | CoNi-LDH/ PEDOT:PSS | 960 (2) 804 (30) | ― | [ |
NiCoAl-LDH/rGO | 1544 (1) 1081 (40) | ― | [ | depositing/growing on conductive substrates+ expanding interlayer distance | |||
NiAl-LDH/NF | 1125 (1) | 819 (200) | [ | ||||
NiFe-LDH/rGO | 1196 (1) 861 (10) | ― | [ | sub-nanometer-scale fine regulation of interlayer distance | |||
NiCo-LDH/C | 2558 (1) 1916 (20) | ― | [ | NiCo-LDH | 2115 (1) 949 (50) | 626 (100) 410 (150) | [ |
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