有机框架膜在气体分离中的研究进展

doi:10.11949/0438-1157.20210269

化工学报 ›› 2021, Vol. 72 ›› Issue (7): 3488-3510.DOI: 10.11949/0438-1157.20210269

有机框架膜在气体分离中的研究进展

王绍宇^1,²(),马翰泽^1,²(),吴洪^1,²,梁旭^1,²,王洪建^1,²,朱姿亭^1,²,姜忠义^1,^2,³()

^1.天津大学化工学院绿色化学化工教育部重点实验室，天津 300072
^2.天津化学化工协同创新中心，天津 300072
^3.天津大学-新加坡国立大学福州联合学院，天津大学福州国际校区，福建福州 350207

收稿日期:2021-02-19 修回日期:2021-04-25 出版日期:2021-07-05 发布日期:2021-07-05
通讯作者: 姜忠义
作者简介:王绍宇(1998—)，男，硕士研究生，shaoyuw_20@tju.edu.cn|马翰泽(1998—)，男，硕士研究生，mahanze@tju.edu.cn
基金资助:
国家自然科学基金项目(21621004);高等学校学科创新引智计划2.0(BP0618007)

Research advances of organic framework membranes in gas separation

WANG Shaoyu^1,²(),MA Hanze^1,²(),WU Hong^1,²,LIANG Xu^1,²,WANG Hongjian^1,²,ZHU Ziting^1,²,JIANG Zhongyi^1,^2,³()

^1.Key Laboratory for Green Technology, School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, China
^2.Collaborative Innovation Center of Chemical Science and Engineering (Tianjin), Tianjin 300072, China
^3.Joint School of National University of Singapore and Tianjin University, International Campus of Tianjin University, Fuzhou 350207, Fujian, China

Received:2021-02-19 Revised:2021-04-25 Online:2021-07-05 Published:2021-07-05
Contact: JIANG Zhongyi

摘要/Abstract

摘要：

高渗透性、高选择性和高稳定性的膜材料是决定膜分离过程效率的关键。有机框架膜（organic framework membranes，OFMs）具有孔隙率高、孔道长程有序、易于官能化修饰、稳定性强等特点，在气体膜分离领域具有重要发展前景。综述了有机框架膜的化学组成、结构特征、制备方法及其在二氧化碳捕集与分离、烯烃/烷烃分离及稀有气体分离等气体分离过程中的应用。最后，对有机框架膜在气体分离领域的机遇和挑战进行了总结，并对其发展方向进行了展望。

关键词: 有机框架膜, 膜分离, 气体分离, 多孔材料, 膜制备方法

Abstract:

Materials with high permeability, high selectivity and high stability are the critical factors to efficient membrane separation processes. Organic framework membranes (OFMs) hold great prospects in gas separation, owing to their high porosity, long-range regular structure, facilely-tailored functionality, and high stability. This review summarized the chemical compositions, structures, fabrications of OFMs and their applications in carbon dioxide capture and separation, olefin/paraffin separation and noble gas separation. Finally, the major challenges and brief perspectives of OFMs in gas separation are tentatively identified.

Key words: organic framework membrane, membrane separation, gas separation, porous materials, fabrication of membrane

中图分类号:

TQ 028.8

王绍宇, 马翰泽, 吴洪, 梁旭, 王洪建, 朱姿亭, 姜忠义. 有机框架膜在气体分离中的研究进展[J]. 化工学报, 2021, 72(7): 3488-3510.

WANG Shaoyu, MA Hanze, WU Hong, LIANG Xu, WANG Hongjian, ZHU Ziting, JIANG Zhongyi. Research advances of organic framework membranes in gas separation[J]. CIESC Journal, 2021, 72(7): 3488-3510.

图/表 6

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有机框架膜在气体分离中的研究进展

Research advances of organic framework membranes in gas separation

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