CIESC Journal ›› 2021, Vol. 72 ›› Issue (3): 1230-1241.DOI: 10.11949/0438-1157.20200855
• Reviews and monographs • Previous Articles Next Articles
TANG Heli1(),ZHANG Bing1(),HUANG Dongmei1,SHEN Yu1,2(),GAO Xu1,2,SHI Wenxin3
Received:
2020-06-30
Revised:
2020-09-21
Online:
2021-03-05
Published:
2021-03-05
Contact:
ZHANG Bing,SHEN Yu
唐和礼1(),张冰1(),黄冬梅1,申渝1,2(),高旭1,2,时文歆3
通讯作者:
张冰,申渝
作者简介:
唐和礼(1998—),男,硕士研究生,基金资助:
CLC Number:
TANG Heli, ZHANG Bing, HUANG Dongmei, SHEN Yu, GAO Xu, SHI Wenxin. Advances in membrane fouling analysis based on XDLVO theory[J]. CIESC Journal, 2021, 72(3): 1230-1241.
唐和礼, 张冰, 黄冬梅, 申渝, 高旭, 时文歆. XDLVO理论在膜污染解析中的应用研究[J]. 化工学报, 2021, 72(3): 1230-1241.
污染物-膜材料 | 前期阶段 | 后期阶段 | ||||||||
---|---|---|---|---|---|---|---|---|---|---|
ΔGLW/ (mJ·m-2) | ΔGAB/ (mJ·m-2) | ΔGEL/ (mJ·m-2) | ΔGTOT/ (mJ·m-2) | MFI×10-3 | ΔGLW/ (mJ·m-2) | ΔGAB/(mJ·m-2) | ΔGEL/(mJ·m-2) | ΔGTOT/(mJ·m-2) | MFI×10-3 | |
TiO2-PES | -5.79 | 24.52 | 0.21 | 18.94 | 3.58 | -11.45 | 25.16 | 0.24 | 13.95 | 1.78 |
(2 mg/L HA-TiO2)-PES | -5.81 | 23.75 | 0.21 | 18.15 | 8.23 | -11.52 | 24.31 | 0.25 | 13.04 | 3.48 |
(3 mg/L HA-TiO2)-PES | -5.70 | 22.35 | 0.17 | 16.82 | 11.7 | -11.10 | 21.76 | 0.30 | 10.96 | 3.67 |
(5 mg/L HA-TiO2)-PES | -5.62 | 22.06 | 0.03 | 16.47 | 20.7 | -10.80 | 21.20 | 0.39 | 10.79 | 4.91 |
(10 mg/L HA-TiO2)-PES | -5.61 | 20.13 | -0.02 | 14.50 | 27.6 | -10.75 | 17.32 | 0.41 | 6.98 | 5.86 |
MFI(×10-3)-ΔGTOT线性拟合 | y = -5.49x + 107.6, R2 = 0.93 | y = -0.53x + 9.8, R2 = 0.84 | ||||||||
TiO2-PVDF | -7.02 | -13.14 | 0.05 | 20.11 | 3.53 | -11.45 | 25.16 | 0.24 | 13.95 | 2.37 |
(2 mg/L HA-TiO2) -PVDF | -7.04 | -16.89 | 0.05 | -23.90 | 8.78 | -11.52 | 24.31 | 0.25 | 13.04 | 6.29 |
(3 mg/L HA-TiO2)-PVDF | -6.92 | -19.36 | 0.03 | -26.37 | 12.0 | -11.10 | 21.76 | 0.30 | 10.96 | 6.79 |
(5 mg/L HA-TiO2)-PVDF | -6.82 | -20.29 | -0.09 | -27.47 | 21.2 | -10.80 | 21.20 | 0.39 | 10.79 | 9.51 |
(10 mg/L HA-TiO2)-PVDF | -6.80 | -23.30 | -0.36 | -30.54 | 19.0 | -10.75 | 17.32 | 0.41 | 6.98 | 10.8 |
MFI×10-3 -ΔGTOT线性拟合 | y = 1.68x - 30.3, R2 = 0.82 | y = -1.07x + 19.1, R2 = 0.78 |
Table 1 Adhesion interfacial free energies in different phases of membrane filtration with HA-TiO2 and the correlativity of ΔGTOT and membrane fouling index[32]
污染物-膜材料 | 前期阶段 | 后期阶段 | ||||||||
---|---|---|---|---|---|---|---|---|---|---|
ΔGLW/ (mJ·m-2) | ΔGAB/ (mJ·m-2) | ΔGEL/ (mJ·m-2) | ΔGTOT/ (mJ·m-2) | MFI×10-3 | ΔGLW/ (mJ·m-2) | ΔGAB/(mJ·m-2) | ΔGEL/(mJ·m-2) | ΔGTOT/(mJ·m-2) | MFI×10-3 | |
TiO2-PES | -5.79 | 24.52 | 0.21 | 18.94 | 3.58 | -11.45 | 25.16 | 0.24 | 13.95 | 1.78 |
(2 mg/L HA-TiO2)-PES | -5.81 | 23.75 | 0.21 | 18.15 | 8.23 | -11.52 | 24.31 | 0.25 | 13.04 | 3.48 |
(3 mg/L HA-TiO2)-PES | -5.70 | 22.35 | 0.17 | 16.82 | 11.7 | -11.10 | 21.76 | 0.30 | 10.96 | 3.67 |
(5 mg/L HA-TiO2)-PES | -5.62 | 22.06 | 0.03 | 16.47 | 20.7 | -10.80 | 21.20 | 0.39 | 10.79 | 4.91 |
(10 mg/L HA-TiO2)-PES | -5.61 | 20.13 | -0.02 | 14.50 | 27.6 | -10.75 | 17.32 | 0.41 | 6.98 | 5.86 |
MFI(×10-3)-ΔGTOT线性拟合 | y = -5.49x + 107.6, R2 = 0.93 | y = -0.53x + 9.8, R2 = 0.84 | ||||||||
TiO2-PVDF | -7.02 | -13.14 | 0.05 | 20.11 | 3.53 | -11.45 | 25.16 | 0.24 | 13.95 | 2.37 |
(2 mg/L HA-TiO2) -PVDF | -7.04 | -16.89 | 0.05 | -23.90 | 8.78 | -11.52 | 24.31 | 0.25 | 13.04 | 6.29 |
(3 mg/L HA-TiO2)-PVDF | -6.92 | -19.36 | 0.03 | -26.37 | 12.0 | -11.10 | 21.76 | 0.30 | 10.96 | 6.79 |
(5 mg/L HA-TiO2)-PVDF | -6.82 | -20.29 | -0.09 | -27.47 | 21.2 | -10.80 | 21.20 | 0.39 | 10.79 | 9.51 |
(10 mg/L HA-TiO2)-PVDF | -6.80 | -23.30 | -0.36 | -30.54 | 19.0 | -10.75 | 17.32 | 0.41 | 6.98 | 10.8 |
MFI×10-3 -ΔGTOT线性拟合 | y = 1.68x - 30.3, R2 = 0.82 | y = -1.07x + 19.1, R2 = 0.78 |
污染物-膜材料 | 前期阶段 | 后期阶段 | 文献 | ||||||
---|---|---|---|---|---|---|---|---|---|
ΔGLW/(mJ·m-2) | ΔGAB/ (mJ·m-2) | ΔGEL/(mJ·m-2) | ΔGTOT/ (mJ·m-2) | ΔGLW/(mJ·m-2) | ΔGAB/ (mJ·m-2) | ΔGEL/(mJ·m-2) | ΔGTOT/ (mJ·m-2) | ||
polystyrene-Al2O3 | -3.45 | -32.54 | 1.16×10-6 | -35.99 | -6.56 | -80.82 | 2.55×10-6 | -87.38 | [ |
glass-Al2O3 | -2.16 | 5.55 | 6.27×10-7 | 23.39 | -2.58 | 44.37 | 8.72×10-6 | 41.78 | [ |
SiO2-PAN | -4.66 | -0.589 | 5.67×10-10 | -5.25 | -2.81 | 9.39 | 5.87×10-10 | 6.58 | [ |
TiO2-PES | -5.79 | 24.52 | 0.21 | 18.94 | -11.45 | 25.16 | 0.24 | 13.95 | [ |
TiO2-PVDF | -7.02 | -13.14 | 0.05 | 20.11 | -11.45 | 25.16 | 0.24 | 13.95 | [ |
SA-PVDF | 1.83 | -19.65 | -0.10 | -17.82 | -3.34 | 12.09 | 0.27 | 8.74 | [ |
SA-PES | -3.38 | 17.12 | -0.04 | 13.75 | -3.34 | 12.09 | 0.27 | 8.74 | [ |
BSA-PVDF | 2.03 | -9.31 | 0.08 | -7.21 | -4.13 | 17.60 | 0.09 | 13.56 | [ |
BSA-PES | -4.20 | 21.14 | -0.52 | 16.43 | -4.13 | 17.60 | 0.09 | 13.56 | [ |
HA-PVDF① | 33.17 | 620.21 | 49.47 | 702.85 | -27.35 | 1717.42 | 3.30 | 1693.37 | [ |
HA-PES① | -56.14 | 2512.99 | 101.38 | 2558.23 | -27.35 | 1717.42 | 3.30 | 1693.37 | [ |
(HA+BSA)-PES① | -31.62 | 221.98 | 51.71 | 241.78 | -20.37 | -162.22 | 5.70 | -176.85 | [ |
(SiO2-NOM)-PES① | -97.98 | -362.55 | 87.70 | -372.83 | -42.15 | -141.38 | 5.81 | -177.72 | [ |
污泥絮体-PVDF | -3.80 | -20.44 | 0.16 | -24.08 | -7.47 | -28.56 | 0.12 | -35.92 | [ |
HPO-混合纤维素 | -4.69 | -51.35 | -0.65 | -56.69 | -3.45 | -72.35 | 0.02 | -75.78 | [ |
TPI-混合纤维素 | -5.53 | -38.45 | -0.53 | 44.51 | -4.79 | -39.98 | 0.02 | -44.75 | [ |
C-HPI-混合纤维素 | -3.70 | 32.63 | -0.33 | 28.60 | -2.15 | 35.56 | 0.04 | 33.45 | [ |
N-HPI-混合纤维素 | -4.34 | -47.95 | -0.80 | -53.10 | -2.96 | -60.04 | 0.01 | -62.99 | [ |
酱油-PVDF(0.45②) | -7.64 | 15.72 | -4.83×10-6 | 8.07 | -5.70 | 25.27 | 4.72×10-10 | 19.87 | [ |
酱油-PES(0.45②) | -0.44 | -1.27 | -8.72×10-7 | -1.71 | -5.70 | 25.27 | 4.72×10-10 | 19.87 | [ |
Table 2 Adhesion interfacial free energies in different phases of membrane filtration with different foulants
污染物-膜材料 | 前期阶段 | 后期阶段 | 文献 | ||||||
---|---|---|---|---|---|---|---|---|---|
ΔGLW/(mJ·m-2) | ΔGAB/ (mJ·m-2) | ΔGEL/(mJ·m-2) | ΔGTOT/ (mJ·m-2) | ΔGLW/(mJ·m-2) | ΔGAB/ (mJ·m-2) | ΔGEL/(mJ·m-2) | ΔGTOT/ (mJ·m-2) | ||
polystyrene-Al2O3 | -3.45 | -32.54 | 1.16×10-6 | -35.99 | -6.56 | -80.82 | 2.55×10-6 | -87.38 | [ |
glass-Al2O3 | -2.16 | 5.55 | 6.27×10-7 | 23.39 | -2.58 | 44.37 | 8.72×10-6 | 41.78 | [ |
SiO2-PAN | -4.66 | -0.589 | 5.67×10-10 | -5.25 | -2.81 | 9.39 | 5.87×10-10 | 6.58 | [ |
TiO2-PES | -5.79 | 24.52 | 0.21 | 18.94 | -11.45 | 25.16 | 0.24 | 13.95 | [ |
TiO2-PVDF | -7.02 | -13.14 | 0.05 | 20.11 | -11.45 | 25.16 | 0.24 | 13.95 | [ |
SA-PVDF | 1.83 | -19.65 | -0.10 | -17.82 | -3.34 | 12.09 | 0.27 | 8.74 | [ |
SA-PES | -3.38 | 17.12 | -0.04 | 13.75 | -3.34 | 12.09 | 0.27 | 8.74 | [ |
BSA-PVDF | 2.03 | -9.31 | 0.08 | -7.21 | -4.13 | 17.60 | 0.09 | 13.56 | [ |
BSA-PES | -4.20 | 21.14 | -0.52 | 16.43 | -4.13 | 17.60 | 0.09 | 13.56 | [ |
HA-PVDF① | 33.17 | 620.21 | 49.47 | 702.85 | -27.35 | 1717.42 | 3.30 | 1693.37 | [ |
HA-PES① | -56.14 | 2512.99 | 101.38 | 2558.23 | -27.35 | 1717.42 | 3.30 | 1693.37 | [ |
(HA+BSA)-PES① | -31.62 | 221.98 | 51.71 | 241.78 | -20.37 | -162.22 | 5.70 | -176.85 | [ |
(SiO2-NOM)-PES① | -97.98 | -362.55 | 87.70 | -372.83 | -42.15 | -141.38 | 5.81 | -177.72 | [ |
污泥絮体-PVDF | -3.80 | -20.44 | 0.16 | -24.08 | -7.47 | -28.56 | 0.12 | -35.92 | [ |
HPO-混合纤维素 | -4.69 | -51.35 | -0.65 | -56.69 | -3.45 | -72.35 | 0.02 | -75.78 | [ |
TPI-混合纤维素 | -5.53 | -38.45 | -0.53 | 44.51 | -4.79 | -39.98 | 0.02 | -44.75 | [ |
C-HPI-混合纤维素 | -3.70 | 32.63 | -0.33 | 28.60 | -2.15 | 35.56 | 0.04 | 33.45 | [ |
N-HPI-混合纤维素 | -4.34 | -47.95 | -0.80 | -53.10 | -2.96 | -60.04 | 0.01 | -62.99 | [ |
酱油-PVDF(0.45②) | -7.64 | 15.72 | -4.83×10-6 | 8.07 | -5.70 | 25.27 | 4.72×10-10 | 19.87 | [ |
酱油-PES(0.45②) | -0.44 | -1.27 | -8.72×10-7 | -1.71 | -5.70 | 25.27 | 4.72×10-10 | 19.87 | [ |
膜材料名称 | γ- /(mJ·m–2) | ζ /mV | ΔG121 /(mJ·m-2) | 文献 | |||
---|---|---|---|---|---|---|---|
改性膜 | 基膜 | 改性膜 | 基膜 | 改性膜 | 基膜 | ||
PVDF/PES/PVA | 27.58 | 13.91 | -25.0 | -29.35 | 0.51 | -28.32 | [ |
PVDF-HEA | 30.13 | 10.48 | -30.83 | -20.95 | 5.24 | -36.92 | [ |
PES-PVP | 4.23 | 0.47 | — | — | -47.13 | -77.49 | [ |
PES-PVP-GO | 13.39 | 0.47 | — | — | -21.08 | -77.49 | [ |
PAN-PAMAM-ETA/NAOH | 52.70 | 7.67 | — | — | 22.55 | -6.14 | [ |
PVDF@ZnO (100 cycles) | 12.4 | 0.6 | -20.7 | -13.7 | — | — | [ |
PVDF@ZnO (200 cycles) | 46.3 | 0.6 | -27.8 | -13.7 | — | — | [ |
PA/Fe@PVDF-OH | 42.34 | 14.65 | -24.24 | -18.40 | — | — | [ |
PVDF@(TiO2/PSS)7 | 19.6 | 0.53 | -39.4 | -20.3 | — | — | [ |
PES-Ni@TiO2 | 44.188 | 7.098 | -35.74 | -33.8 | — | — | [ |
PANI-DBSA | 48.7 | 19.6 | -55.0 | -40.3 | — | — | [ |
PVDF-GO-Ni | 63.04 | 22.59 | -5.95 | -13.38 | — | — | [ |
Table 3 The key properties of modified membranes
膜材料名称 | γ- /(mJ·m–2) | ζ /mV | ΔG121 /(mJ·m-2) | 文献 | |||
---|---|---|---|---|---|---|---|
改性膜 | 基膜 | 改性膜 | 基膜 | 改性膜 | 基膜 | ||
PVDF/PES/PVA | 27.58 | 13.91 | -25.0 | -29.35 | 0.51 | -28.32 | [ |
PVDF-HEA | 30.13 | 10.48 | -30.83 | -20.95 | 5.24 | -36.92 | [ |
PES-PVP | 4.23 | 0.47 | — | — | -47.13 | -77.49 | [ |
PES-PVP-GO | 13.39 | 0.47 | — | — | -21.08 | -77.49 | [ |
PAN-PAMAM-ETA/NAOH | 52.70 | 7.67 | — | — | 22.55 | -6.14 | [ |
PVDF@ZnO (100 cycles) | 12.4 | 0.6 | -20.7 | -13.7 | — | — | [ |
PVDF@ZnO (200 cycles) | 46.3 | 0.6 | -27.8 | -13.7 | — | — | [ |
PA/Fe@PVDF-OH | 42.34 | 14.65 | -24.24 | -18.40 | — | — | [ |
PVDF@(TiO2/PSS)7 | 19.6 | 0.53 | -39.4 | -20.3 | — | — | [ |
PES-Ni@TiO2 | 44.188 | 7.098 | -35.74 | -33.8 | — | — | [ |
PANI-DBSA | 48.7 | 19.6 | -55.0 | -40.3 | — | — | [ |
PVDF-GO-Ni | 63.04 | 22.59 | -5.95 | -13.38 | — | — | [ |
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