化工学报 ›› 2024, Vol. 75 ›› Issue (4): 1167-1182.DOI: 10.11949/0438-1157.20231127
申州洋(), 薛康(), 刘青, 史成香, 邹吉军, 张香文, 潘伦()
收稿日期:
2023-11-01
修回日期:
2024-01-04
出版日期:
2024-04-25
发布日期:
2024-06-06
通讯作者:
薛康,潘伦
作者简介:
申州洋(1999—),男,硕士研究生,szy_0315@tju.edu.cn
基金资助:
Zhouyang SHEN(), Kang XUE(), Qing LIU, Chengxiang SHI, Jijun ZOU, Xiangwen ZHANG, Lun PAN()
Received:
2023-11-01
Revised:
2024-01-04
Online:
2024-04-25
Published:
2024-06-06
Contact:
Kang XUE, Lun PAN
摘要:
吸热型纳米流体燃料是一种有潜力解决高超声速飞行器发动机过热问题的新型燃料。为探究吸热型纳米流体燃料的裂解性能,并为后续研究提供参考,首先介绍了纳米流体燃料的分散稳定性机理,并概述了其制备及提高稳定性的方法;其次,综述了吸热型纳米流体燃料的裂解研究进展,从纳米添加剂、有机保护配体及反应机理和路径等多方面分析了影响裂解的关键因素;最后对吸热型纳米流体燃料的未来发展趋势提出展望。
中图分类号:
申州洋, 薛康, 刘青, 史成香, 邹吉军, 张香文, 潘伦. 吸热型纳米流体燃料研究进展[J]. 化工学报, 2024, 75(4): 1167-1182.
Zhouyang SHEN, Kang XUE, Qing LIU, Chengxiang SHI, Jijun ZOU, Xiangwen ZHANG, Lun PAN. Research progress on endothermic nanofluid fuels[J]. CIESC Journal, 2024, 75(4): 1167-1182.
图3 纳米颗粒的布朗运动(a)和DLVO理论与纳米流体稳定性(b)示意图[23-25]
Fig.3 Schematic diagram of Brownian motion of nanoparticles (a) and DLVO theory and nanofluid stability (b)[23-25]
图4 0.5% GO浓度的JP-10静置0 h(a)、3 h(b)、和2周(c)时的照片[41]
Fig.4 Photographs of GO dispersed at a concentration of 0.5% in JP-10 with different time: (a) 0 h; (b) 3 h; (c) 2 weeks[41]
图5 (a)Pt@FGS提高n-C12H26分解机理示意图;(b)Pt@FGS表面H2生成和Pt团簇复原的分子动力学示意图(青色:碳;白色:氢;红色:氧;橙色:铂)[59]
Fig.5 (a) Schematic of the proposed enhancing mechanisms of n-C12H26 fuel decomposition in the presence of Pt@FGS;(b) MD snapshots for an example of H2 formation from the surface of Pt@FGS and the recovery of Pt-cluster on the FGS (cyan: C, white: H, red: O, and orange: Pt)[59]
图7 超支化聚甘油(HMS)[61](a),超支化聚乙烯亚胺(HPEI)[50](b)和超支化聚合物包覆金属纳米颗粒协同催化十氢萘裂解的示意图[40](c)
Fig.7 Schematic of hyperbranched polyglycerol (HMS)[61] (a), hyperbranched polyethyleneimine (HPEI)[50] (b), and the synergistic catalytic cracking of decalin by hyperbranched poly(amidoamine)-encapsulated metal nanoparticles (HEMNs)[40] (c)
文献 | 纳米颗粒 | 燃料基液 | 温度/℃ | 压力/MPa | 转化率/% | 热沉/(MJ/kg) |
---|---|---|---|---|---|---|
[ | 钯 | 十氢萘 | 750 | 3.50 | 91.9 | 3.50 |
[ | 铂 | JP-10 | 680 | 4.00 | 55.2 | 2.70 |
[ | 铂 | 十氢萘 | 675 | 3.50 | 50.7 | 2.62 |
[ | 钯 | 十氢萘 | 725 | 4.00 | 77.0 | 3.61 |
[ | 铂 | 甲基环己烷 | 650 | 3.50 | 33.0 | 2.24 |
[ | 铂 | 甲基环己烷 | 650 | 3.50 | 61.5 | 2.39 |
表1 贵金属纳米流体燃料裂解性能
Table 1 Cracking performance of precious metal nanofluid fuels
文献 | 纳米颗粒 | 燃料基液 | 温度/℃ | 压力/MPa | 转化率/% | 热沉/(MJ/kg) |
---|---|---|---|---|---|---|
[ | 钯 | 十氢萘 | 750 | 3.50 | 91.9 | 3.50 |
[ | 铂 | JP-10 | 680 | 4.00 | 55.2 | 2.70 |
[ | 铂 | 十氢萘 | 675 | 3.50 | 50.7 | 2.62 |
[ | 钯 | 十氢萘 | 725 | 4.00 | 77.0 | 3.61 |
[ | 铂 | 甲基环己烷 | 650 | 3.50 | 33.0 | 2.24 |
[ | 铂 | 甲基环己烷 | 650 | 3.50 | 61.5 | 2.39 |
文献 | 纳米颗粒 | 燃料基液 | 温度/℃ | 压力/MPa | 转化率/% | 热沉/(MJ/kg) |
---|---|---|---|---|---|---|
[ | Beta分子筛 | JP-10 | 700 | 4.00 | 63.2 | 2.80 |
[ | ZSM-5 | 正癸烷 | 758 | 3.00 | — | 4.64 |
表2 分子筛纳米流体燃料裂解性能
Table 2 Cracking performance of molecular sieve nanofluid fuels
文献 | 纳米颗粒 | 燃料基液 | 温度/℃ | 压力/MPa | 转化率/% | 热沉/(MJ/kg) |
---|---|---|---|---|---|---|
[ | Beta分子筛 | JP-10 | 700 | 4.00 | 63.2 | 2.80 |
[ | ZSM-5 | 正癸烷 | 758 | 3.00 | — | 4.64 |
图11 ReaxFF-MD模拟得到含氧FGS催化脱氢的反应路径:(a)去质子化/质子化,(b)再生,(c)1700 K下含有FGS的MCH保持6.0 ns的反应路径[90]
Fig.11 Reaction pathways for catalytic dehydrogenation by the oxygen-containing FGS, derived by ReaxFF MD simulations: (a) deprotonation/protonation, (b) regeneration, (c) reaction pathways for MCH containing added FGS held at 1700 K for 6.0 ns[90]
文献 | 纳米颗粒 | 燃料基液 | 温度/℃ | 压力/MPa | 转化率/% | 热沉/(MJ/kg) |
---|---|---|---|---|---|---|
[ | Pt@FGS | JP-10 | 420 | 4.00 | 48.5 | — |
[ | FGS | 甲基环己烷 | 547 | 4.70 | 64.2 | — |
表3 石墨烯纳米流体燃料裂解性能
Table 3 Cracking performance of graphene nanofluid fuels
文献 | 纳米颗粒 | 燃料基液 | 温度/℃ | 压力/MPa | 转化率/% | 热沉/(MJ/kg) |
---|---|---|---|---|---|---|
[ | Pt@FGS | JP-10 | 420 | 4.00 | 48.5 | — |
[ | FGS | 甲基环己烷 | 547 | 4.70 | 64.2 | — |
图13 C-十一烷基杯[4]烃间苯二酚分子结构示意图(a); C-十一烷基杯[4]烃间苯二酚包覆镍纳米颗粒(b)和Ni-B非晶合金(c)的TEM图[93-94]
Fig.13 Molecular structure of C-undecyl calix[4]resorcinarene (a); TEM images of C-undecyl calix[4]resorcinarene-encapsulated Ni nanoparticles (b) and Ni-B nano-amorphous alloy (c)[93-94]
文献 | 纳米颗粒 | 燃料基液 | 温度/℃ | 压力/MPa | 转化率/% | 热沉/(MJ/kg) |
---|---|---|---|---|---|---|
[ | Ni/SiO2-A | 正癸烷 | 750 | 3.50 | 84.0 | 3.93 |
[ | Ni/SiO2 | 正癸烷 | 750 | 3.50 | — | 4.04 |
[ | ZSM-5@NiM | 正癸烷 | 780 | 3.00 | — | 4.59 |
表4 过渡金属纳米流体燃料裂解性能
Table 4 Cracking performance of transition metal nanofluid fuels
文献 | 纳米颗粒 | 燃料基液 | 温度/℃ | 压力/MPa | 转化率/% | 热沉/(MJ/kg) |
---|---|---|---|---|---|---|
[ | Ni/SiO2-A | 正癸烷 | 750 | 3.50 | 84.0 | 3.93 |
[ | Ni/SiO2 | 正癸烷 | 750 | 3.50 | — | 4.04 |
[ | ZSM-5@NiM | 正癸烷 | 780 | 3.00 | — | 4.59 |
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