化工学报 ›› 2023, Vol. 74 ›› Issue (4): 1735-1745.DOI: 10.11949/0438-1157.20221646

• 能源和环境工程 • 上一篇    下一篇

余热回收喷淋塔的烟气颗粒物脱除特性研究

时国华1,2(), 何林珅1, 赵玺灵3(), 张世钢4   

  1. 1.华北电力大学动力工程系,河北 保定 071003
    2.华北电力大学河北省低碳高效发电技术重点实验室,河北 保定 071003
    3.清华大学建筑学院,北京 100084
    4.北京清建能源技术有限公司,北京 100085
  • 收稿日期:2022-12-29 修回日期:2023-03-14 出版日期:2023-04-05 发布日期:2023-06-02
  • 通讯作者: 时国华,赵玺灵
  • 作者简介:时国华(1980—),男,博士,副教授,lucksgh@126.com
  • 基金资助:
    北京市科技计划项目(Z191100009119005)

Study of removal characteristics of particulate matters within flue gas by spray tower for waste-heat recovery

Guohua SHI1,2(), Linshen HE1, Xiling ZHAO3(), Shigang ZHANG4   

  1. 1.Department of Power Engineering, North China Electric Power University, Baoding 071003, Hebei, China
    2.Hebei Key Laboratory of Low Carbon and High Efficiency Power Generation Technology, North China Electric Power University, Baoding 071003, Hebei, China
    3.School of Architecture, Tsinghua University, Beijing 100084, China
    4.Beijing Qingjian Energy Technology Co. , Ltd. , Beijing 100085, China
  • Received:2022-12-29 Revised:2023-03-14 Online:2023-04-05 Published:2023-06-02
  • Contact: Guohua SHI, Xiling ZHAO

摘要:

喷淋塔喷淋低温水可回收烟气余热和净化烟气。以喷淋塔为研究对象,建立喷淋塔内气-液热质交换、颗粒物异质凝结增长与脱除模型,探究余热回收喷淋塔内烟气颗粒物脱除机理,研究不同工况下颗粒物脱除特性。结果表明:当烟气入口温度50℃、入口相对湿度100%、水气比2 L/m³、喷淋水温20℃、喷淋水滴粒径550 μm时,在喷淋塔下半部区域,水滴主要靠热泳与扩散泳捕集亚微米级颗粒物;随着水蒸气在亚微米级颗粒物表面凝结,在喷淋塔上部区域,惯性碰撞为水滴捕集亚微米级颗粒物的主要机制。提高水气比、降低喷淋水温、减小液滴粒径、增大气液两相温差及水汽饱和度均可提高喷淋塔内颗粒物脱除效率,其中水气比为2.5 L/m3,喷淋水温为10~15℃,可实现较好的颗粒物脱除效果。

关键词: 喷淋塔, 颗粒物, 凝结, 烟道气, 捕集

Abstract:

The low-temperature water sprayed by the spray tower can recover the waste heat of the flue gas and purify the flue gas. In the study, the models evaluating the heat and mass exchange between flue gas and water drops, the size growth of particulate matters (PMs) caused by heterogeneous condensation and the removal of PMs in the spray tower were developed to explore the mechanisms of removing PMs within coal-fired flue gas coupled with waste heat recovery. The removal characteristics of PMs in the flue gas were also investigated under various working conditions of the spray tower. The results show that the capture mechanisms of sub-micrometer PMs in the lower part of the spray tower are mainly thermophoresis and diffusiophoresis while the capture mechanism of sub-micrometer PMs in the upper part of the spray tower is inertial collision due to water vapor condensed on the sub-micrometer PMs at the flue gas inlet temperature of 50℃, the flue gas inlet relative humidity of 100%, the water- gas ratio of 2 L/m³, the cold water temperature of 20℃, and the spray water droplet size of 550 μm. For the spray tower, the removal efficiency of PMs can be improved under the conditions of higher water-gas ratios, lower spray water temperatures, lower water droplet sizes, and higher temperature differences between flue gas and water droplets, or higher water vapor saturation levels. The spray tower has the better removal performance of PMs at the condition of water-gas ratio of 2.5 L/m3 and spray water temperatures of 10—15℃.

Key words: spray tower, particulate matter, condensation, flue gas, capture

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