化工学报 ›› 2014, Vol. 65 ›› Issue (1): 55-60.DOI: 10.3969/j.issn.0438-1157.2014.01.007

• 流体力学与传递现象 • 上一篇    下一篇

微通道中气体/离子液体两相流动与分散性能

谭璟, 赵菁菁, 徐建鸿, 骆广生   

  1. 清华大学化学工程系, 化学工程联合国家重点实验室, 北京 100084
  • 收稿日期:2013-07-01 修回日期:2013-11-01 出版日期:2014-01-05 发布日期:2014-01-05
  • 通讯作者: 骆广生
  • 作者简介:谭璟(1984-),女,博士。
  • 基金资助:

    国家自然科学基金项目(21206081,21036002);博士后科学基金项目(02320101076)。

Flow and dispersion performance of gas/ionic liquid systems in microchannels

TAN Jing, ZHAO Jingjing, XU Jianhong, LUO Guangsheng   

  1. State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China
  • Received:2013-07-01 Revised:2013-11-01 Online:2014-01-05 Published:2014-01-05
  • Supported by:

    supported by the National Natural Science Foundation of China(21206081, 21036002).

摘要: 离子液体在气-液反应与分离过程中有良好的应用前景,研究气体/离子液体两相体系的微分散过程对于发展新型气-液分散技术和设备具有重要意义。研究了N2/[Bmim]BF4体系在同轴环管微通道中的流动和分散行为。实验结果表明,在不同的气相和液相流速下,N2/[Bmim]BF4体系分别呈现气泡流、气泡-气柱过渡流、气柱流和气柱-环隙流过渡流4种流型。通过考察分散相尖端尺寸和气相、液相流速对气-液体系流型的影响,作出了相应的流型图。通过考察气相、液相流速对稳定气-液分散流型下的气相分散尺寸的影响,揭示了分散气相行为的机理,并建立了描述气相分散尺寸的数学模型。

关键词: 微通道, 气-液体系, 离子液体, 分散

Abstract: Ionic liquids show good prospect in gas-liquid reaction and separation processes. Investigation of flow and dispersion performance of gas/ionic liquid systems is important for the development of technology and devices for gas-liquid dispersion as well as application of ionic liquids in gas-liquid reaction and separation processes. The flow and dispersion performance of N2/[Bmim]BF4 in coaxial annular microchannels was investigated. Flow patterns of bubble-flow, bubble-slug-transition-flow, slug-flow and slug-annular-transition-flow were observed. The influence of gas and liquid flow rates on gas-liquid flow pattern was studied in different microchannels and flow pattern maps were determined accordingly. The effects of gas and liquid flow rates on dispersion size were also investigated. The mechanism was discussed and mathematical models were established to predict the dispersion size in different microchannels.

Key words: microchannel, gas-liquid system, ionic liquids, dispersion

中图分类号: